简介:Onenewsesquiterpenecompound,namely,illihenlactoneA(1),andonenewprenylatedC6–C3compound,illihenryioneH(2),alongwiththreeknownsesquiterpenes(3–5)wereisolatedfromthestemsofIlliciumhenryi.Thestructuresof1and2wereelucidatedbyspectroscopicevidenceincludingNMR,HRESIMSandcirculardichroism(CD).Compound2exhibitedaweakinhibitoryratioforbglucuronidasereleaseinducedbyplatelet-activatingfactor(PAF)inratpolymorphonuclearleukocytes(PMNs)invitro.
简介:Anenvironmentallyfriendlyprecursor,adenosine,hasbeenusedasadualsourceofCandNtosynthesizenitrogen-dopedcarboncatalystwith/withoutFe.Ahydrothermalcarbonizationmethodhasbeenusedandwateristhecarbonizationmedia.Themorphologyofsampleswith/withoutFecomponenthasbeencomparedbyHRTEM,andtheresultshowsthatFecanpromotethegraphitizationofcarbon.Furtherelectro-chemicaltestshowsthattheoxygenreductionreaction(ORR)catalyticactivityofFe-containingsample(C–FeN)ismuchhigherthanthatoftheFe-freesample(C–N).Additionally,theintermediatesofC–FeNformedduringeachsyntheticprocedurehavebeenthoroughlycharacterizedbymultiplemethods,andthefunctionofeachprocedurehasbeendiscussed.TheC–FeNsampleexhibitshighelectro-catalyticstabilityandsuperiorelectro-catalyticactivitytowardORRinalkalinemedia,withitshalf-wavepotential20mVlowerthanthatofcommercialPt/C(40wt%).Itisfurtherincorporatedintoalkalinepolymerelectrolytefuelcell(APEFC)asthecathodematerialandledtoapowerdensityof100mW/cm~2.
简介:Thediscretizationsizeislimitedbythesamplingtheorem,andthelimitisonehalfofthewavelengthofthehighestfrequencyoftheproblem.However,onehalfofthewavelengthisanidealvalue.Ingeneral,thediscretizationsizethatcanensuretheaccuracyofthesimulationismuchsmallerthanthisvalueinthetraditionalfiniteelementmethod.Thepossiblereasonofthisphenomenonisanalyzedinthispaper,andanefficientmethodisgiventoimprovethesimulationaccuracy.
简介:ThisarticledescribesalocalerrorestimatorforGlimm'sschemeforhyperbolicsystemsofconservationlawsandusesittoreplacetheusualrandomchoiceinGlimm'sschemebyanoptimalchoice.Asaby-productofthelocalerrorestimator,theprocedureprovidesaglobalerrorestimatorthatisshownnumericallytobeaveryaccurateestimateoftheerrorinL1(R)foralltimes.Althoughthereispartialmathematicalevidencefortheerrorestimatorproposed,atthisstagetheerrorestimatormustbeconsideredad-hoc.Nonetheless,theerrorestimatorissimpletocompute,relativelyinexpensive,withoutadjustableparametersandatleastasaccurateasotherexistingerrorestimators.Numericalexperimentsin1-DforBurgers'equationandforEuler'ssystemareperformedtomeasuretheasymptoticaccuracyoftheresultingschemeandoftheerrorestimator.
简介:<正>InthepresentnotethealgebraicindependenceofvaluesofseveralMahlerserieswithcertainparticularanddifferentparametersatalgebraicpointsisestablishedbymeansofatypicalapproximationmethodhandlingtheLiouvilletypeseries.
简介:InthispaperwediscusstheconvergenceofamodifiedNewton’smethodpresentedbyA.Ostrowski[1]andJ.F.Traub[2],whichhasquadraticconvergenceorderbutreducesoneevaluationofthederivativeateverytwostepscomparedwithNewton’smethod.Aconvergencetheoremisestablishedbyusingaweakconditiona≤3-2(21/2)andasharperrorestimateisgivenabouttheiterativesequence.
简介:
简介:LetT=(T(t))t≥0beaboundedC-regularizedsemigroupgeneratedbyAonaBanachspaceXandR(C)bedenseinX.WeshowthatifthereisadensesubspaceYofXsuchthatforeveryx∈Y,σu(A,Cx),thesetofallpointsλ∈iRtowhich(λ-A)^-1Cxcannotbeextendedholomorphically,isatmostcountableandσr(A)NiR=Ф,thenTisstable.AstabilityresultforthecaseofR(C)beingnon-denseisalsogiven.Ourresultsgeneralizetheworkonthestabilityofstronglycontinuoussenfigroups.
简介:受非线性增生映射值域的扰动定理的启发,研究了非线性边值问题(@)在L^p(Ω),1<p<+∞中解的存在性。(@){-∑^Ni,j=1σ/σxi(ai,jσu/σxj)+∑^Ni=1bσu/σxi+g(x,u)=fa.e.inΩ,-σu/σna∈βx(u(x))a.e.onΓ其中f∈L^p(Ω),1<p<+∞给定,g:Ω×R→满足Caratheodory条件。本文把Gupta和Hass所研究的非线性方程加以推广,即在方程中增加了∑^Ni=1bσu/σxi这一项,并把解的存在性的讨论由L^2(Ω)空间推广到L^p(Ω),1<p<+∞空间中。
简介:Variousagriculturalcropresiduesincludingcornstover,corncob,andsorghumstalkwithamoisturecontentof75wt%weresubjectedtoalongpretreatment(12-60h)withsupercriticalCO2(scCO2),atlowtemperature(50-80℃)andapressureof17.5-25.0Mpa.Thesugaryieldsfromtheenzymatichydrolysis(EH)ofthepretreatedsampleswereasmuchasthree-tofourfoldgreaterthanthoseaffordedbytherawmaterials.However,whenpretreatmentwasconductedwithinashorttime(e.g.0.5h),aspreviouslyreportedintheliterature,onlyaslightincreaseintheEHsugaryieldswasobserved.TheproposedscCO2pretreatmentmechanismdemonstratedtheroleofmoistureinthesystem.Wetting,softening,andswellingwereobservedtomainlyaffectthelignocellulosewhenasuitableamountofwaterwasadded.Finally,thesampleswereanalysedbyX-raydiffractionandscanningelectronmicroscopy,beforeandafterpretreatment,toinvestigatethechangesinthemicroscopicstructureofthebiomass.